PAPERSPECIFICS OF STUDYFINDINGS Kohler, 1936 (“The nucleus in and the growth of hygroscopic droplets”) Evaporate 2kg of hoar-frost and determined Cl content;

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PAPERSPECIFICS OF STUDYFINDINGS Kohler, 1936 (“The nucleus in and the growth of hygroscopic droplets”) Evaporate 2kg of hoar-frost and determined Cl content; used optics to measure droplet size; thermodynamic analysis to look at condensation [Cl] rain droplet ≅ [Cl] cloud droplet ; d[Cl]/dz < 0; “selection” of droplet size – large ones grow first at expense of smaller Twomey, 1974 (“Pollution and planetary albedo”) Theoretical approach to relate optical thickness to cloud albedo; observed data over several hours from Southeast Australia used to examine effects of pollution on # of cloud nuclei Pollution  addition of cloud nuclei  increase solar reflection; cloud reflectance dominant role in planetary albedo; Albedo α optical thickness (thickness is DOMINANT in determining albedo); # cloud nuclei ↑  optical thickness ↑  increase in reflected solar (net cooling) Albrecht, 1989 (“Aerosols, cloud microphysics, and fractional cloudiness”) Q: How do aerosols affect fractional cloudiness of marine Sc and cumulus? Used optical array probe to estimate droplet concentrations; GOES images to detect ship tracks; Used model simulation to calculate fractional cloud amount Over ocean, ↑ CCN  ↓ droplet size  ↓ drizzle production  ↑ Cloud liquid water and cloudiness. Increase in cloud lifetime leads to increase in reflected solar (net cooling)

PAPERSPECIFICS OF STUDYFINDINGS Lenton & Vaughan, 2009 (“The radiative forcing potential of different climate geoengineering options”) – cited Albrecht, 1989 Theoretical considerations of radiation budgets and radiative transfer Climate geoengineering best considered as COMPLEMENT to mitigation of CO2 emissions, not an ALTERNATIVE; up to -4Wm -2 radiative forcing on century timescale Kazil et al (“Aerosol nucleation and its role for clouds and Earth’s radiative forcing in the aerosol-climate model ECHAM5-HAM”) – cited Twomey, 1974 Used aerosol-climate model ECHAM5-HAM, implemented new scheme for “neutral and charged nucleation” of H 2 SO 4 and H 2 O based on empirical studies Overall radiative effect of nucleation is -2.55Wm -2 (-2.18 over oceans, over land; discrepancy partially due to larger surface area of oceans) Petters & Kreidenweis, 2007 (“A single parameter representation of hygroscopic growth and condensation nucleus activity”) – cited Kohler, 1936 Relate particle dry diameter and CCN activity using “single hygroscopicity parameter” κ; use a modeling approach based on Kohler theory Hygroscopicity parameter can be used to model CCN activity of atmospheric particles

PAPERSPECIFICS OF STUDYFINDINGS Ackerman et al (“Large- Eddy Simulations of a Drizzling, Stratocumulus- Topped Marine Boundary Layer”) – cited Albrecht, 1989 Model simulations initialized by aircraft measurements which measured aerosol concentrations, wind, moisture, etc; comparison of several simulations Mean LWP well reproduced; mean entrainment rate lower; including drizzle leads to decrease in LWP for nearly all model simulations Lohmann et al (“Total aerosol effect: radiative forcing or radiative flux perturbation?”) – cited Twomey, 1974 Attempt to quantify feedbacks induced by interactions of aerosols with clouds and radiation; use “radiative flux perturbations” (RFP) method, using various GCMs Feedbacks and interactions that are fast compared to global warming timescales should be included in anthropogenic feedback estimates;