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Eugene Demler Harvard University
Simulations of strongly correlated electron systems using cold atoms Eugene Demler Harvard University Main collaborators: Anatoli Polkovnikov Harvard/Boston University Ehud Altman Harvard/Weizmann Daw-Wei Wang Harvard/Tsing-Hua University Vladimir Gritsev Harvard Adilet Imambekov Harvard Ryan Barnett Harvard/Caltech Mikhail Lukin Harvard
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Strongly correlated electron systems
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“Conventional” solid state materials
Bloch theorem for non-interacting electrons in a periodic potential
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Consequences of the Bloch theorem
VH EF d Metals I Insulators and Semiconductors EF First semiconductor transistor
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“Conventional” solid state materials
Electron-phonon and electron-electron interactions are irrelevant at low temperatures ky kx Landau Fermi liquid theory: when frequency and temperature are smaller than EF electron systems are equivalent to systems of non-interacting fermions kF Discuss Widemann-Franz law. It works for … Ag Ag Ag
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Non Fermi liquid behavior in novel quantum materials
Violation of the Wiedemann-Franz law in high Tc superconductors Hill et al., Nature 414:711 (2001) UCu3.5Pd1.5 Andraka, Stewart, PRB 47:3208 (93) CeCu2Si2. Steglich et al., Z. Phys. B 103:235 (1997)
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Puzzles of high temperature superconductors
Unusual “normal” state Maple, JMMM 177:18 (1998) Resistivity, opical conductivity, Lack of sharply defined quasiparticles, Nernst effect Mechanism of Superconductivity High transition temperature, retardation effect, isotope effect, role of elecron-electron and electron-phonon interactions Competing orders Role of magnetsim, stripes, possible fractionalization
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Applications of quantum materials: High Tc superconductors
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Applications of quantum materials: Ferroelectric RAM
V _ _ _ _ _ _ _ _ FeRAM in Smart Cards Non-Volatile Memory High Speed Processing
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Modeling strongly correlated
systems using cold atoms
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Bose-Einstein condensation
Cornell et al., Science 269, 198 (1995) Ultralow density condensed matter system Interactions are weak and can be described theoretically from first principles
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New Era in Cold Atoms Research
Focus on Systems with Strong Interactions Atoms in optical lattices Feshbach resonances Low dimensional systems Systems with long range dipolar interactions Rotating systems
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Feshbach resonance and fermionic condensates
Greiner et al., Nature 426:537 (2003); Ketterle et al., PRL 91: (2003) Ketterle et al., Nature 435, (2005)
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One dimensional systems
1D confinement in optical potential Weiss et al., Science (05); Bloch et al., Esslinger et al., One dimensional systems in microtraps. Thywissen et al., Eur. J. Phys. D. (99); Hansel et al., Nature (01); Folman et al., Adv. At. Mol. Opt. Phys. (02) Strongly interacting regime can be reached for low densities
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Atoms in optical lattices
Theory: Jaksch et al. PRL (1998) Experiment: Kasevich et al., Science (2001); Greiner et al., Nature (2001); Phillips et al., J. Physics B (2002) Esslinger et al., PRL (2004); and many more …
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Strongly correlated systems
Electrons in Solids Atoms in optical lattices Simple metals Perturbation theory in Coulomb interaction applies. Band structure methods wotk Strongly Correlated Electron Systems Band structure methods fail. Novel phenomena in strongly correlated electron systems: Quantum magnetism, phase separation, unconventional superconductivity, high temperature superconductivity, fractionalization of electrons …
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New Era in Cold Atoms Research
Focus on Systems with Strong Interactions Goals Resolve long standing questions in condensed matter physics (e.g. origin of high temperature superconductivity) Resolve matter of principle questions (e.g. existence of spin liquids in two and three dimensions) Study new phenomena in strongly correlated systems (e.g. coherent far from equilibrium dynamics)
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Outline Introduction. Cold atoms in optical lattices. Bose Hubbard model Two component Bose mixtures Quantum magnetism. Competing orders. Fractionalized phases Fermions in optical lattices Pairing in systems with repulsive interactions. High Tc mechanism Boson-Fermion mixtures Polarons. Competing orders Interference experiments with fluctuating BEC Analysis of correlations beyond mean-field Moving condensates in optical lattices Non equilibrium dynamics of interacting many-body systems Emphasis: detection and characterzation of many-body states
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Atoms in optical lattices. Bose Hubbard model
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Bose Hubbard model U t tunneling of atoms between neighboring wells
repulsion of atoms sitting in the same well
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Bose Hubbard model. Mean-field phase diagram
M.P.A. Fisher et al., PRB40:546 (1989) N=3 Mott 4 Superfluid N=2 Mott 2 N=1 Mott Superfluid phase Weak interactions Mott insulator phase Strong interactions
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Bose Hubbard model Set Hamiltonian eigenstates are Fock states 2 4
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Bose Hubbard Model. Mean-field phase diagram
Mott 4 Superfluid N=2 Mott 2 N=1 Mott Mott insulator phase Particle-hole excitation Tips of the Mott lobes
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Gutzwiller variational wavefunction
Normalization Interaction energy Kinetic energy z – number of nearest neighbors
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Phase diagram of the 1D Bose Hubbard model. Quantum Monte-Carlo study
Batrouni and Scaletter, PRB 46:9051 (1992)
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Optical lattice and parabolic potential
4 N=2 MI SF 2 N=1 MI Jaksch et al., PRL 81:3108 (1998)
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Superfluid to Insulator transition
Greiner et al., Nature 415:39 (2002) t/U Superfluid Mott insulator What if the ground state cannot be described by single particle matter waves? Current experiments are reaching such regimes. A nice example is the experiment by Markus and collaborators in Munich where cold bosons on an optical lattice were tuned across the SF-Mott transition. Explain experiment. SF well described by a wavefunction in which the zero momentum state is macroscopically occupied. Mott state is rather well described by definite RS occupations.
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Time of flight experiments
Quantum noise interferometry of atoms in an optical lattice Second order coherence
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Second order coherence in the insulating state of bosons
Second order coherence in the insulating state of bosons. Hanburry-Brown-Twiss experiment Theory: Altman et al., PRA 70:13603 (2004) Experiment: Folling et al., Nature 434:481 (2005)
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Hanburry-Brown-Twiss stellar interferometer
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Hanburry-Brown-Twiss interferometer
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Second order coherence in the insulating state of bosons
Bosons at quasimomentum expand as plane waves with wavevectors First order coherence: Oscillations in density disappear after summing over Second order coherence: Correlation function acquires oscillations at reciprocal lattice vectors
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Second order coherence in the insulating state of bosons
Second order coherence in the insulating state of bosons. Hanburry-Brown-Twiss experiment Theory: Altman et al., PRA 70:13603 (2004) Experiment: Folling et al., Nature 434:481 (2005)
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Effect of parabolic potential on the second order coherence
Experiment: Spielman, Porto, et al., Theory: Scarola, Das Sarma, Demler, cond-mat/ Width of the correlation peak changes across the transition, reflecting the evolution of Mott domains
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Width of the noise peaks
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Interference of an array of independent condensates
Hadzibabic et al., PRL 93: (2004) Smooth structure is a result of finite experimental resolution (filtering)
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Extended Hubbard Model
- nearest neighbor repulsion - on site repulsion Checkerboard phase: Crystal phase of bosons. Breaks translational symmetry
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Extended Hubbard model. Mean field phase diagram
van Otterlo et al., PRB 52:16176 (1995) Hard core bosons. Supersolid – superfluid phase with broken translational symmetry
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Extended Hubbard model. Quantum Monte Carlo study
Hebert et al., PRB 65:14513 (2002) Sengupta et al., PRL 94: (2005)
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Dipolar bosons in optical lattices
Goral et al., PRL88: (2002)
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How to detect a checkerboard phase
Correlation Function Measurements
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Magnetism in condensed matter systems
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Ferromagnetism Magnetic needle in a compass
Ferromagnetism is known since the time of the ancient greeks. Magnetic materials find numerous applications Starting from magnetic needle in a compass and including hard drives which can carry terabytes of information. Record holder for commercial products: Hitachi hard drives with density of 230 billion bits per sq. inch. This allows Computer drives capable of storing a trillion bytes (terabyte) Magnetic memory in hard drives. Storage density of hundreds of billions bits per square inch.
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Stoner model of ferromagnetism
Spontaneous spin polarization decreases interaction energy but increases kinetic energy of electrons Our current knowledge does not go beyond the original simple argument by Stoner. Hubbard model for fermions was originally proposed to explain ferromagnetism. After Many years of numerical studies, it is now believed that the Hubbard model does Not have ferromagnetism. And Hubbard model is really the simplest example. When we take systems with more realistic long range interactions, we do not Really know when such mean-field argument applies. For example, there Is currently a lot of controversy and debates regarding possible ferromagnetism in 2d electron gas at low density. I N(0) = 1 Mean-field criterion I – interaction strength N(0) – density of states at the Fermi level
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Antiferromagnetism Maple, JMMM 177:18 (1998) High temperature superconductivity in cuprates is always found near an antiferromagnetic insulating state
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( - ) ( + ) ( + ) Antiferromagnetism t t
Antiferromagnetic Heisenberg model AF = ( ) S = ( ) t = ( ) AF = S t Antiferromagnetic state breaks spin symmetry. It does not have a well defined spin
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Spin liquid states Alternative to classical antiferromagnetic state: spin liquid states Properties of spin liquid states: fractionalized excitations topological order gauge theory description Systems with geometric frustration ?
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Spin liquid behavior in systems with geometric frustration
Kagome lattice Pyrochlore lattice SrCr9-xGa3+xO19 ZnCr2O4 A2Ti2O7 Ramirez et al. PRL (90) Broholm et al. PRL (90) Uemura et al. PRL (94) Ramirez et al. PRL (02)
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Engineering magnetic systems using cold atoms in an optical lattice
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Spin interactions using controlled collisions
Experiment: Mandel et al., Nature 425:937(2003) Theory: Jaksch et al., PRL 82:1975 (1999)
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Effective spin interaction from the orbital motion.
Cold atoms in Kagome lattices Santos et al., PRL 93:30601 (2004) Damski et al., PRL 95:60403 (2005)
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Two component Bose mixture in optical lattice
Example: Mandel et al., Nature 425:937 (2003) t t Two component Bose Hubbard model
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Quantum magnetism of bosons in optical lattices
Kuklov and Svistunov, PRL (2003) Duan et al., PRL (2003) Ferromagnetic Antiferromagnetic
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Exchange Interactions in Solids
antibonding bonding Kinetic energy dominates: antiferromagnetic state Coulomb energy dominates: ferromagnetic state
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Two component Bose mixture in optical lattice
Two component Bose mixture in optical lattice. Mean field theory + Quantum fluctuations Altman et al., NJP 5:113 (2003) Hysteresis 1st order 2nd order line
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Coherent spin dynamics in optical lattices
Widera et al., cond-mat/ atoms in the F=2 state
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How to observe antiferromagnetic order of cold atoms in an optical lattice?
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Second order coherence in the insulating state of bosons
Second order coherence in the insulating state of bosons. Hanburry-Brown-Twiss experiment Theory: Altman et al., PRA 70:13603 (2004) See also Bach, Rzazewski, PRL 92: (2004) Experiment: Folling et al., Nature 434:481 (2005) See also Hadzibabic et al., PRL 93: (2004)
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Probing spin order of bosons
Correlation Function Measurements
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Engineering exotic phases
Optical lattice in 2 or 3 dimensions: polarizations & frequencies of standing waves can be different for different directions YY ZZ Example: exactly solvable model Kitaev (2002), honeycomb lattice with Can be created with 3 sets of standing wave light beams ! Non-trivial topological order, “spin liquid” + non-abelian anyons …those has not been seen in controlled experiments
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Fermionic atoms in optical lattices
Pairing in systems with repulsive interactions. Unconventional pairing. High Tc mechanism
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Fermionic atoms in a three dimensional optical lattice
Kohl et al., PRL 94:80403 (2005)
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Fermions with attractive interaction
Hofstetter et al., PRL 89: (2002) U t t Highest transition temperature for Compare to the exponential suppresion of Tc w/o a lattice
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Reaching BCS superfluidity in a lattice
Turning on the lattice reduces the effective atomic temperature K in NdYAG lattice 40K Li in CO2 lattice 6Li Superfluidity can be achived even with a modest scattering length
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Fermions with repulsive interactions
Possible d-wave pairing of fermions
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High temperature superconductors
Picture courtesy of UBC Superconductivity group High temperature superconductors Superconducting Tc 93 K Hubbard model – minimal model for cuprate superconductors P.W. Anderson, cond-mat/ After many years of work we still do not understand the fermionic Hubbard model
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Positive U Hubbard model
Possible phase diagram. Scalapino, Phys. Rep. 250:329 (1995) Antiferromagnetic insulator D-wave superconductor
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Second order correlations in the BCS superfluid
n(k) n(r) n(r’) k F k BCS BEC
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Momentum correlations in paired fermions
Greiner et al., PRL 94: (2005)
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Fermion pairing in an optical lattice
Second Order Interference In the TOF images Normal State Superfluid State measures the Cooper pair wavefunction One can identify unconventional pairing
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Boson Fermion mixtures
Fermions interacting with phonons. Polarons. Competing orders
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Boson Fermion mixtures
Experiments: ENS, Florence, JILA, MIT, Rice, … BEC Bosons provide cooling for fermions and mediate interactions. They create non-local attraction between fermions Charge Density Wave Phase Periodic arrangement of atoms Non-local Fermion Pairing P-wave, D-wave, …
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Boson Fermion mixtures
“Phonons” : Bogoliubov (phase) mode Effective fermion-”phonon” interaction Fermion-”phonon” vertex Similar to electron-phonon systems
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Boson Fermion mixtures in 1d optical lattices
Cazalila et al., PRL (2003); Mathey et al., PRL (2004) Spinless fermions Spin ½ fermions Note: Luttinger parameters can be determined using correlation function measurements in the time of flight experiments. Altman et al. (2005)
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BF mixtures in 2d optical lattices
Wang, Lukin, Demler, PRA (1972) 40K -- 87Rb 40K -- 23Na (a) =1060nm =1060 nm (b) =765.5nm
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Systems of cold atoms with strong interactions and correlations
Goals Resolve long standing questions in condensed matter physics (e.g. origin of high temperature superconductivity) Resolve matter of principle questions (e.g. existence of spin liquids in two and three dimensions) Study new phenomena in strongly correlated systems Interference experiments with fluctuating BEC Analysis of high order correlation functions in low dimensional systems Moving condensates in optical lattices Non equilibrium dynamics of interacting many-body systems
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Interference experiments with fluctuating BEC
Analysis of high order correlation functions in low dimensional systems
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Interference of two independent condensates
Andrews et al., Science 275:637 (1997)
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Interference of two independent condensates
1 r+d d 2 Clouds 1 and 2 do not have a well defined phase difference. However each individual measurement shows an interference pattern
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Interference of one dimensional condensates
Experiments: Schmiedmayer et al., Nature Physics (2005) d Amplitude of interference fringes, , contains information about phase fluctuations within individual condensates x1 x2 y x
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Interference amplitude and correlations
Polkovnikov, Altman, Demler, PNAS (2006) L For identical condensates Instantaneous correlation function
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Interference between Luttinger liquids
Luttinger liquid at T=0 L K – Luttinger parameter For non-interacting bosons and For impenetrable bosons and Luttinger liquid at finite temperature Analysis of can be used for thermometry
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Rotated probe beam experiment
For large imaging angle, , Luttinger parameter K may be extracted from the angular dependence of q
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Interference between two-dimensional
BECs at finite temperature. Kosteritz-Thouless transition
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Interference of two dimensional condensates
Experiments: Stock, Hadzibabic, Dalibard, et al., cond-mat/ Gati, Oberthaler, et al., cond-mat/ Lx Ly Lx Probe beam parallel to the plane of the condensates
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Interference of two dimensional condensates
Interference of two dimensional condensates. Quasi long range order and the KT transition Ly Lx Theory: Polkovnikov, Altman, Demler, PNAS (2006) Above KT transition Below KT transition
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Experiments with 2D Bose gas
Haddzibabic et al., Nature (2006) z Time of flight x Typical interference patterns low temperature higher temperature
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Experiments with 2D Bose gas
Hadzibabic et al., Nature (2006) x z integration over x axis integration distance Dx (pixels) Contrast after integration 0.4 0.2 10 20 30 middle T z low T high T integration over x axis z integration over x axis Dx z
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Experiments with 2D Bose gas
Hadzibabic et al., Nature (2006) 0.4 0.2 10 20 30 low T middle T high T fit by: Integrated contrast Exponent a central contrast 0.5 0.1 0.2 0.3 0.4 high T low T “Sudden” jump!? integration distance Dx if g1(r) decays exponentially with : if g1(r) decays algebraically or exponentially with a large :
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Experiments with 2D Bose gas
Hadzibabic et al., Nature (2006) Exponent a T (K) 1.0 1.1 1.2 c.f. Bishop and Reppy 0.5 0.1 0.2 0.3 0.4 high T low T central contrast Ultracold atoms experiments: jump in the correlation function. KT theory predicts a=1/4 just below the transition He experiments: universal jump in the superfluid density
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Experiments with 2D Bose gas
Experiments with 2D Bose gas. Proliferation of thermal vortices Haddzibabic et al., Nature (2006) 10% 20% 30% central contrast 0.1 0.2 0.3 0.4 high T low T Fraction of images showing at least one dislocation Exponent a 0.5 0.1 0.2 0.3 0.4 central contrast The onset of proliferation coincides with a shifting to 0.5! Z. Hadzibabic et al., Nature (2006)
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Full distribution function of the interference amplitude
Interference between two interacting one dimensional Bose liquids Full distribution function of the interference amplitude Gritsev, Altman, Demler, Polkovnikov, cond-mat/
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Higher moments of interference amplitude
is a quantum operator. The measured value of will fluctuate from shot to shot. Can we predict the distribution function of ? Higher moments Changing to periodic boundary conditions (long condensates) Explicit expressions for are available but cumbersome Fendley, Lesage, Saleur, J. Stat. Phys. 79:799 (1995)
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Impurity in a Luttinger liquid
Expansion of the partition function in powers of g Partition function of the impurity contains correlation functions taken at the same point and at different times. Moments of interference experiments come from correlations functions taken at the same time but in different points. Euclidean invariance ensures that the two are the same
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Relation between quantum impurity problem and interference of fluctuating condensates
Normalized amplitude of interference fringes Distribution function of fringe amplitudes Relation to the impurity partition function Distribution function can be reconstructed from using completeness relations for the Bessel functions
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Bethe ansatz solution for a quantum impurity
can be obtained from the Bethe ansatz following Zamolodchikov, Phys. Lett. B 253:391 (91); Fendley, et al., J. Stat. Phys. 79:799 (95) Making analytic continuation is possible but cumbersome Interference amplitude and spectral determinant is related to the single particle Schroedinger equation Dorey, Tateo, J.Phys. A. Math. Gen. 32:L419 (1999) Bazhanov, Lukyanov, Zamolodchikov, J. Stat. Phys. 102:567 (2001) Spectral determinant
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Evolution of the distribution function
Narrow distribution for Approaches Gumble distribution. Width Wide Poissonian distribution for
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From interference amplitudes to conformal field theories
correspond to vacuum eigenvalues of Q operators of CFT Bazhanov, Lukyanov, Zamolodchikov, Comm. Math. Phys.1996, 1997, 1999 When K>1, is related to Q operators of CFT with c<0. This includes 2D quantum gravity, non-intersecting loop model on 2D lattice, growth of random fractal stochastic interface, high energy limit of multicolor QCD, … Yang-Lee singularity 2D quantum gravity, non-intersecting loops on 2D lattice
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Moving condensates in optical lattices
Non equilibrium coherent dynamics of interacting many-body systems
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Atoms in optical lattices. Bose Hubbard model
Theory: Jaksch et al. PRL 81:3108(1998) Experiment: Kasevich et al., Science (2001) Greiner et al., Nature (2001) Cataliotti et al., Science (2001) Phillips et al., J. Physics B (2002) Esslinger et al., PRL (2004), …
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Equilibrium superfluid to insulator transition
Theory: Fisher et al. PRB (89), Jaksch et al. PRL (98) Experiment: Greiner et al. Nature (01) U m Superfluid Mott insulator What if the ground state cannot be described by single particle matter waves? Current experiments are reaching such regimes. A nice example is the experiment by Markus and collaborators in Munich where cold bosons on an optical lattice were tuned across the SF-Mott transition. Explain experiment. SF well described by a wavefunction in which the zero momentum state is macroscopically occupied. Mott state is rather well described by definite RS occupations. t/U
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Moving condensate in an optical lattice. Dynamical instability
Theory: Niu et al. PRA (01), Smerzi et al. PRL (02) Experiment: Fallani et al. PRL (04) v Related experiments by Eiermann et al, PRL (03)
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??? This discussion: How to connect
the dynamical instability (irreversible, classical) to the superfluid to Mott transition (equilibrium, quantum) Unstable ??? p U/J p/2 Stable SF MI This discussion U/t p SF MI ??? Possible experimental sequence:
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Superconductor to Insulator transition in thin films
Marcovic et al., PRL 81:5217 (1998) Bi films d Superconducting films of different thickness
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Dynamical instability
Classical limit of the Hubbard model. Discreet Gross-Pitaevskii equation Current carrying states Linear stability analysis: States with p>p/2 are unstable Amplification of density fluctuations unstable unstable r
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Dynamical instability for integer filling
Order parameter for a current carrying state Current GP regime Maximum of the current for When we include quantum fluctuations, the amplitude of the order parameter is suppressed decreases with increasing phase gradient
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Dynamical instability for integer filling
SF MI p U/J p/2 Vicinity of the SF-I quantum phase transition. Classical description applies for The amplitude and the phase of the order parameter can only be defined if we coarse grain the system on the scale ksi. Applying the same argument as before we find the condition that p ksi should be of the order of pi over two. Near the SF-I transition ksi diverges. So the critical phase gradient goes to zero. Dynamical instability occurs for
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Dynamical instability. Gutzwiller approximation
Wavefunction Time evolution We look for stability against small fluctuations Phase diagram. Integer filling
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Optical lattice and parabolic trap. Gutzwiller approximation
The first instability develops near the edges, where N=1 U=0.01 t J=1/4 Gutzwiller ansatz simulations (2D)
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Beyond semiclassical equations. Current decay by tunneling
phase j phase j phase j Current carrying states are metastable. They can decay by thermal or quantum tunneling Thermal activation Quantum tunneling
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Decay of current by quantum tunneling
phase j phase Quantum phase slip j Escape from metastable state by quantum tunneling. WKB approximation S – classical action corresponding to the motion in an inverted potential.
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Decay rate from a metastable state. Example
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For d>1 we have to include transverse directions.
Need to excite many chains to create a phase slip Longitudinal stiffness is much smaller than the transverse. The transverse size of the phase slip diverges near a phase slip. We can use continuum approximation to treat transverse directions
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Weakly interacting systems. Gross-Pitaevskii regime.
Decay of current by quantum tunneling SF MI p U/J p/2 Fallani et al., PRL (04) Quantum phase slips are strongly suppressed in the GP regime
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Strongly interacting regime. Vicinity of the SF-Mott transition
MI p U/J p/2 Close to a SF-Mott transition we can use an effective relativistivc GL theory (Altman, Auerbach, 2004) Metastable current carrying state: This state becomes unstable at corresponding to the maximum of the current:
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Strongly interacting regime. Vicinity of the SF-Mott transition
Decay of current by quantum tunneling SF MI p U/J p/2 Action of a quantum phase slip in d=1,2,3 - correlation length Strong broadening of the phase transition in d=1 and d=2 is discontinuous at the transition. Phase slips are not important. Sharp phase transition
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Decay of current by quantum tunneling
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Decay of current by thermal activation
phase j phase Thermal phase slip j DE Escape from metastable state by thermal activation
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Thermally activated current decay. Weakly interacting regime
phase slip DE Activation energy in d=1,2,3 Thermal fluctuations lead to rapid decay of currents Crossover from thermal to quantum tunneling
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Decay of current by thermal fluctuations
Phys. Rev. Lett. (2004)
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Conclusions We understand well: electron systems in semiconductors and simple metals. Interaction energy is smaller than the kinetic energy. Perturbation theory works We do not understand: strongly correlated electron systems in novel materials. Interaction energy is comparable or larger than the kinetic energy. Many surprising new phenomena occur, including high temperature superconductivity, magnetism, fractionalization of excitations Ultracold atoms have energy scales of 10-6K, compared to 104 K for electron systems. However, by engineering and studying strongly interacting systems of cold atoms we should get insights into the mysterious properties of novel quantum materials Our big goal is to develop a general framework for understanding strongly correlated systems. This will be important far beyond AMO and condensed matter
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