Ondřej Svoboda Nuclear Physics Institute, Academy of Sciences of Czech Republic Department of Nuclear Reactors, Faculty of Nuclear Sciences and Physical.

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Determination of experimental cross-sections by activation method
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Presentation transcript:

Ondřej Svoboda Nuclear Physics Institute, Academy of Sciences of Czech Republic Department of Nuclear Reactors, Faculty of Nuclear Sciences and Physical Engineering, Czech Technical University in Prague Cross-section measurements of the (n,xn) threshold reactions 1.6 GeV deuteron irradiation of the Energy plus Transmutation setup

Outline Motivation for  measurementsMotivation for  measurements Requirements for  measurementsRequirements for  measurements TSL Uppsala experimentTSL Uppsala experiment Experiments on Cyclotron in ŘežExperiments on Cyclotron in Řež Cross-section conclusionCross-section conclusion 1.6 GeV deuteron E+T experiment1.6 GeV deuteron E+T experiment Simulations and comparisons of Exp × SimSimulations and comparisons of Exp × Sim Data share spaceData share space E+T conclusionE+T conclusion - Motivation for  measurements - Requirements - TSL Uppsala - Cyclotron Řež -  conclusion - E+T:1.6 GeV d+ - Simulations & comparisons - Data share - E+T conclusion

Motivation for  measurement – E+T - Motivation for  measurements Energy plus Transmutation Yield to neutron flux - Requirements - TSL Uppsala - Cyclotron Řež -  conclusion - E+T:1.6 GeV d+ - Simulations & comparisons - Data share - E+T conclusion

We want to measure Yield to neutron flux problem Solving a Fredholm equation we can find Φ(E): Solving a Fredholm equation we can find Φ(E): We would like to find! (Up to know only MCNPX simulation) Poor knowledge of  Measured in E+T - Motivation for  measurements Energy plus Transmutation Yield to neutron flux - Requirements - TSL Uppsala - Cyclotron Řež -  conclusion - E+T:1.6 GeV d+ - Simulations & comparisons - Data share - E+T conclusion

Requirements for  -measurements by activation method: - high energy neutron source with good intensity - (quasi)monoenergetic neutrons with well known spectrum - pure monoisotopic samples - good spectroscopic equipment –  and X-rays spectrometers - knowledge about the corrections on beam fluctuation, self- absorption, non-point like emitters… Requirements for  measurements Evaluation process: Irradiation HPGe Spectra evaluation Corrections N Yield - Motivation for  measurements - Requirements Equipment Materials - TSL Uppsala - Cyclotron Řež -  conclusion - E+T:1.6 GeV d+ - Simulations & comparisons - Data share - E+T conclusion

Measured materials Reaction E thresh [MeV] Half-life 197 Au (n,2n) 196 Au d 197 Au (n,3n) 195 Au d d 197 Au (n,4n) 194 Au h 197 Au (n,5n) 193 Au h 197 Au (n,6n) 192 Au h 197 Au (n,7n) 191 Au h In Řež also measured: Mg, Ni, Fe, Zn iodine (KIO 4 ) - Motivation for  measurements - Requirements Equipment Materials - TSL Uppsala - Cyclotron Řež -  conclusion - E+T:1.6 GeV d+ - Simulations & comparisons - Data share - E+T conclusion

TSL Uppsala - Protons on Li target or spallation source - Neutrons with energies MeV - Well known beam and neutron spectrum - Motivation for  measurements - Requirements - TSL Uppsala Introduction Blue hall Experiment Measurements - Cyclotron Řež -  conclusion - E+T:1.6 GeV d+ - Simulations & comparisons - Data share - E+T conclusion

TSL Uppsala – Blue hall - Motivation for  measurements - Requirements - TSL Uppsala Introduction Blue hall Experiment Measurements - Cyclotron Řež -  conclusion - E+T:1.6 GeV d+ - Simulations & comparisons - Data share - E+T conclusion Experimental setup in the Blue hall Neutron spectra

TSL Uppsala - irradiations - 3 irradiations on the Li target – 25, 50, and 100 MeV p+ - Motivation for  measurements - Requirements - TSL Uppsala Introduction Blue hall Experiment Measurements - Cyclotron Řež -  conclusion - E+T:1.6 GeV d+ - Simulations & comparisons - Data share - E+T conclusion June 2008, supported by EFNUDAT program - one irradiation on the ANITA spallation target – 180 MeV p+ Proton beam energy [MeV]24.68 ± ± ± 0.3 Li-target thickness [mm]248.5 Proton beam current [  A] 10 5 Average energy of peak neutrons [MeV] Fraction of neutrons in the peak [%] Peak neutron flux density [10 5 cm -2 s -1 ]

TSL Uppsala – spectroscopic measurements - 8 hours each irradiation - one day of spectroscopic measurements after each irradiation Au, Al, Bi, In, Ta, I samples Present status: Finished yields evaluation, waiting for the beam data... to be completed soon - Motivation for  measurements - Requirements - TSL Uppsala Introduction Blue hall Experiment Measurements - Cyclotron Řež -  conclusion - E+T:1.6 GeV d+ - Simulations & comparisons - Data share - E+T conclusion

Cyclotron Řež - Protons on Li target - Neutrons with energies MeV - Good intensities: 10 8 n cm -2 s -1 - Well equipped spectroscopic laboratory (NSD-NPI) - Motivation for  measurements - Requirements - TSL Uppsala - Cyclotron Řež Introduction Experiments Preliminary results -  conclusion - E+T:1.6 GeV d+ - Simulations & comparisons - Data share - E+T conclusion Beam-line Li-target Graphite stopper Samples

Cyclotron Řež – experiments - Up to now 2 experiments: 20 and 25 MeV - Au, Al, Bi, In, Ta, I, Ni, Fe, Mg, Zn - next irradiations planned on October Motivation for  measurements - Requirements - TSL Uppsala - Cyclotron Řež Introduction Experiments Preliminary results -  conclusion - E+T:1.6 GeV d+ - Simulations & comparisons - Data share - E+T conclusion

Cyclotron Řež – experimental results Tentative data! Evaluation not yet ready… Number of neutrons in peak 196 Au 194 Au - Motivation for  measurements - Requirements - TSL Uppsala - Cyclotron Řež Introduction Experiments Preliminary results -  conclusion - E+T:1.6 GeV d+ - Simulations & comparisons - Data share - E+T conclusion

Conclusion – cross-sections –Uppsala and Řež cross-section measurements covered wide spectrum of energies ( MeV) –Preliminary results show we are close to known cross-section values –Near future – finalize experiment analysis – next experiments at Řež – next experiments at Řež –Farther future – next experiments at Uppsala – application of the results on the E+T experiments – application of the results on the E+T experiments – publish the measured cross-sections with respect to be involved in the EXFOR library if possible – publish the measured cross-sections with respect to be involved in the EXFOR library if possible - Motivation for  measurements - Requirements - TSL Uppsala - Cyclotron Řež -  conclusion - E+T:1.6 GeV d+ - Simulations & comparisons - Data share - E+T conclusion

Energy plus Transmutation - setup Povray code – renders pictures from input files - Motivation for  measurements - Requirements - TSL Uppsala - Cyclotron Řež -  conclusion - E+T:1.6 GeV d+ Setup - videos Longitudinal results Radial results Spectral index d x p – longitud d x p - radial - Simulations & comparisons - Data share - E+T conclusion

Longitudinal distributions of isotopes – at 3 cm produced in Au, Al, Bi and In foils, 1.6 GeV deuterons produced in Au, Al, Bi and In foils, 1.6 GeV deuterons - Motivation for  measurements - Requirements - TSL Uppsala - Cyclotron Řež -  conclusion - E+T:1.6 GeV d+ Setup - videos Longitudinal results Radial results Spectral index d x p – longitud d x p - radial - Simulations & comparisons - Data share - E+T conclusion

Radial distributions of isotopes – 1st gap produced in Au, Al, Bi and In foils, 1.6 GeV deuterons produced in Au, Al, Bi and In foils, 1.6 GeV deuterons - Motivation for  measurements - Requirements - TSL Uppsala - Cyclotron Řež -  conclusion - E+T:1.6 GeV d+ Setup - videos Longitudinal results Radial results Spectral index d x p – longitud d x p - radial - Simulations & comparisons - Data share - E+T conclusion

Spectral index Au/ 196 Au Spectral index 192 Au/ 196 Au Beam - Motivation for  measurements - Requirements - TSL Uppsala - Cyclotron Řež -  conclusion - E+T:1.6 GeV d+ Setup - videos Longitudinal results Radial results Spectral index d x p – longitud d x p - radial - Simulations & comparisons - Data share - E+T conclusion

Comparison between experiments - longitudinal 198 Au 196 Au Yields normalized to the second foil in each experiment - Motivation for  measurements - Requirements - TSL Uppsala - Cyclotron Řež -  conclusion - E+T:1.6 GeV d+ Setup - videos Longitudinal results Radial results Spectral index d x p – longitud d x p - radial - Simulations & comparisons - Data share - E+T conclusion Experiment 198 Au yield x GeV p0.7 ± GeV d3.3 ± GeV d3.8 ± 0.3

Comparison between experiments - radial 198 Au 196 Au Yields normalized to the first foil in each experiment - Motivation for  measurements - Requirements - TSL Uppsala - Cyclotron Řež -  conclusion - E+T:1.6 GeV d+ Setup - videos Longitudinal results Radial results Spectral index d x p – longitud d x p - radial - Simulations & comparisons - Data share - E+T conclusion

Simulations – MCNPX 2.6.E - different INC+evaporation models available - only INCL4+ABLA can simulate deuterons with E > 2 GeV - Motivation for  measurements - Requirements - TSL Uppsala - Cyclotron Řež -  conclusion - E+T:1.6 GeV d+ - Simulations & comparisons MCNPX 2.6.E longitudinal radial - Data share - E+T conclusion But INCL4+ABLA needs 10x more time => solved thanks CESNET METAcentrum

Exp versus Sim – longitudinal - 3 cm over the target axis cm over the target axis - Motivation for  measurements - Requirements - TSL Uppsala - Cyclotron Řež -  conclusion - E+T:1.6 GeV d+ - Simulations & comparisons MCNPX 2.6.E longitudinal radial - Data share - E+T conclusion

Exp versus Sim - radial - first gap - behind the target - Motivation for  measurements - Requirements - TSL Uppsala - Cyclotron Řež -  conclusion - E+T:1.6 GeV d+ - Simulations & comparisons MCNPX 2.6.E longitudinal radial - Data share - E+T conclusion

Data share - Exact setup description in the codes - MCNPX, FLUKA, TALYS - Huge computing power - CESNET We can simulate various problems We offer help and space for collecting your E+T results, perform calculations and make comparisons within the collaboration!! - Motivation for  measurements - Requirements - TSL Uppsala - Cyclotron Řež -  conclusion - E+T:1.6 GeV d+ - Simulations & comparisons - Data share - E+T conclusion

Energy plus Transmutation - conclusion –Analysis of previous E+T experiments finished, simulations performed –Published JINR preprints: E – 1 GeV p E – MC simulations E – 1.5 GeV p –Preprints 0.7 & 2 GeV p, 2.52 & 1.6 GeV d will follow –In October – defense of Antonín Krása PhD. thesis –Future plans: Next E+T experiments – this November?Next E+T experiments – this November? Further cross-section measurementsFurther cross-section measurements Application of measured cross-section data to E+T dataApplication of measured cross-section data to E+T data Thank you for your attention.. - Motivation for  measurements - Requirements - TSL Uppsala - Cyclotron Řež -  conclusion - E+T:1.6 GeV d+ - Simulations & comparisons - Data share - E+T conclusion